Jolie and Pitt were reportedly planning to adopt 2-year-old Syrian boy Moussa from the Altinozu refugee camp in Turkey.
Jolie was said to have met the boy during one of her humanitarian projects in the refugee camp as UN ambassador.
However, sources close to the famous couple told People that the rumors are “totally false” and “absolutely not true.”
Jolie, 39, was in the spotlight last month when she revealed that she had made the decision to remove her ovaries and fallopian tubes after learning she was carrying a cancer gene.
Two years ago she announced that she underwent a double mastectomy to reduce her chances of developing cancer.
Angelina and Brad are already parents to Vivienne and Knox, 6, Shiloh, 8, Zahara, 9, Pax, 11, Maddox, 13.